The collection consists of Neyland's personal files, photographs, correspondence, newspaper clippings, an autobiographical manuscript of his college days, service records, scrapbooks, and yearbooks. Possibly most interesting are 2 ledgers containing Neyland's handwritten notes on various teams, hand-diagrammed plays, notes on player progress and other fascinating insights into his coaching style.

These two photograph album scrapbooks contain images of the three Luther boys - Edwin, Lawrence, Albert - their sister, Louise, and many of their friends during their youth in the 1920s.