The collection consists of Neyland's personal files, photographs, correspondence, newspaper clippings, an autobiographical manuscript of his college days, service records, scrapbooks, and yearbooks. Possibly most interesting are 2 ledgers containing Neyland's handwritten notes on various teams, hand-diagrammed plays, notes on player progress and other fascinating insights into his coaching style.

The Johnny Majors Collection contains material relating to Majors' tenure as a football coach at the University of Tennessee, Knoxville. Spanning from 1983-1993, the collection includes correspondence, playbooks, and assorted athletic files.